Clean Ar-Me conversion to Ar-aldehyde with the aid of carefully designed metallocorrole photocatalysts

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Toluene,p-xylene and mesitylene were cleanly converted to their corresponding monoaldehydesviamild photooxygenation utilizing transition metal and main group beta-CF3-substituted corroles. Aldehyde yield increased as more electron-donating CH(3)groups are present on the substrate.4-Pwas most efficient (TON similar to 1072, mesitylene)viathe singlet oxygen vis the superoxide mechanism.
Publisher
ROYAL SOC CHEMISTRY
Issue Date
2020-08
Language
English
Article Type
Article
Citation

PHOTOCHEMICAL & PHOTOBIOLOGICAL SCIENCES, v.19, no.8, pp.996 - 1000

ISSN
1474-905X
DOI
10.1039/d0pp00218f
URI
http://hdl.handle.net/10203/281937
Appears in Collection
CH-Journal Papers(저널논문)
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