Ferroelectric properties of heteroepitaxial PbTiO3 and PbZr1-xTixO3 films on Nb-doped SrTiO3 fabricated by hydrothermal epitaxy below Curie temperature

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PbTiO3 (PTO) and PbZr1-xTixO3 (PZT) films on a (100) Nb-doped SrTiO3 (NSTO) substrate were fabricated at 160 and 210 degrees C, respectively, by hydrothermal epitaxy below the Curie temperature, T-C. The PTO capacitor had a square hysteresis curve compared to the rounded hysteresis curve of the PZT capacitor. These differing behaviors in the polarization-electric hysteresis curves can be explained by the existence of an interfacial layer formed between the PZT film and the NSTO substrate. The PZT capacitor showed almost no polarization fatigue after 10(11) switching cycles. However, the PTO capacitor revealed a slightly different fatigue behavior due to the microvoids that formed as a result of the agglomeration of the island growth mode. However, the fatigue behavior of both capacitors revealed that defects, such as the lead or oxygen vacancies, were suppressed by the hydrothermal epitaxy using a very low fabrication temperature below T-C.
Publisher
MATERIALS RESEARCH SOC
Issue Date
2007-04
Language
English
Article Type
Article
Keywords

PB(ZR,TI)O3 THIN-FILMS; SINGLE-CRYSTAL; FATIGUE; DOMAIN; HETEROSTRUCTURES; INSTABILITY; ELECTRODES; CAPACITORS; DEPOSITION

Citation

JOURNAL OF MATERIALS RESEARCH, v.22, no.4, pp.1037 - 1042

ISSN
0884-2914
DOI
10.1557/jmr.2007.0122
URI
http://hdl.handle.net/10203/87979
Appears in Collection
MS-Journal Papers(저널논문)
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