Synthesis of alpha-Aminoacetals via Decarboxylative Coupling of Imine and 2,2,-Diethoxyacetic Acid

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dc.contributor.authorKim, Seoksunko
dc.contributor.authorPark, Beomsoonko
dc.contributor.authorLee, Geun Seokko
dc.contributor.authorHong, Soon Hyeokko
dc.date.accessioned2023-06-22T07:00:33Z-
dc.date.available2023-06-22T07:00:33Z-
dc.date.created2022-11-28-
dc.date.created2022-11-28-
dc.date.issued2023-05-
dc.identifier.citationJOURNAL OF ORGANIC CHEMISTRY, v.88, no.10, pp.6532 - 6537-
dc.identifier.issn0022-3263-
dc.identifier.urihttp://hdl.handle.net/10203/308062-
dc.description.abstractAtom-economical C-C coupling between imines and a C1 source could provide alpha-aminoaldehyde derivatives. Nevertheless, such a coupling has rarely been achieved owing to the lack of appropriate nucleophilic C1 sources. In this study, photocatalytic synthesis of alpha-aminoacetals was achieved via decarboxylative coupling of imine and 2,2-diethoxyacetic acid using a nonstoichiometric amount of a radical initiator. Various functional groups were compatible, providing efficient one-step access to diversely functionalized alpha-aminoacetals, which provides a promising platform for further research.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleSynthesis of alpha-Aminoacetals via Decarboxylative Coupling of Imine and 2,2,-Diethoxyacetic Acid-
dc.typeArticle-
dc.identifier.wosid000883922300001-
dc.identifier.scopusid2-s2.0-85141711773-
dc.type.rimsART-
dc.citation.volume88-
dc.citation.issue10-
dc.citation.beginningpage6532-
dc.citation.endingpage6537-
dc.citation.publicationnameJOURNAL OF ORGANIC CHEMISTRY-
dc.identifier.doi10.1021/acs.joc.2c01941-
dc.contributor.localauthorHong, Soon Hyeok-
dc.contributor.nonIdAuthorKim, Seoksun-
dc.contributor.nonIdAuthorLee, Geun Seok-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusLIGHT PHOTOREDOX CATALYSIS-
dc.subject.keywordPlusRADICAL-ADDITION-
dc.subject.keywordPlusAMINO ALDEHYDE-
dc.subject.keywordPlusACETALS-
dc.subject.keywordPlusREACTIVITY-
dc.subject.keywordPlusAMINATION-
dc.subject.keywordPlusCHEMISTRY-
dc.subject.keywordPlusOXIDATION-
dc.subject.keywordPlusUMPOLUNG-
dc.subject.keywordPlusSALTS-
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