DC Field | Value | Language |
---|---|---|
dc.contributor.author | Liu, Bin | ko |
dc.contributor.author | Sun, Huiliang | ko |
dc.contributor.author | Lee, Jin-Woo | ko |
dc.contributor.author | Jiang, Zhengyan | ko |
dc.contributor.author | Qiao, Junqin | ko |
dc.contributor.author | Wang, Junwei | ko |
dc.contributor.author | Yang, Jie | ko |
dc.contributor.author | Feng, Kui | ko |
dc.contributor.author | Liao, Qiaogan | ko |
dc.contributor.author | An, Mingwei | ko |
dc.contributor.author | Li, Bolin | ko |
dc.contributor.author | Han, Dongxue | ko |
dc.contributor.author | Xu, Baomin | ko |
dc.contributor.author | Lian, Hongzhen | ko |
dc.contributor.author | Niu, Li | ko |
dc.contributor.author | Kim, Bumjoon J. | ko |
dc.contributor.author | Guo, Xugang | ko |
dc.date.accessioned | 2023-06-18T06:00:12Z | - |
dc.date.available | 2023-06-18T06:00:12Z | - |
dc.date.created | 2023-06-15 | - |
dc.date.created | 2023-06-15 | - |
dc.date.issued | 2023-02 | - |
dc.identifier.citation | NATURE COMMUNICATIONS, v.14, no.1 | - |
dc.identifier.issn | 2041-1723 | - |
dc.identifier.uri | http://hdl.handle.net/10203/307316 | - |
dc.description.abstract | Degradation of the kinetically trapped bulk heterojunction film morphology in organic solar cells (OSCs) remains a grand challenge for their practical application. Herein, we demonstrate highly thermally stable OSCs using multicomponent photoactive layer synthesized via a facile one-pot polymerization, which show the advantages of low synthetic cost and simplified device fabrication. The OSCs based on multicomponent photoactive layer deliver a high power conversion efficiency of 11.8% and exhibit excellent device stability for over 1000 h (>80% of their initial efficiency retention), realizing a balance between device efficiency and operational lifetime for OSCs. In-depth opto-electrical and morphological properties characterizations revealed that the dominant PM6-b-L15 block polymers with backbone entanglement and the small fraction of PM6 and L15 polymers synergistically contribute to the frozen fine-tuned film morphology and maintain well-balanced charge transport under long-time operation. These findings pave the way towards the development of low-cost and long-term stable OSCs. | - |
dc.language | English | - |
dc.publisher | NATURE PORTFOLIO | - |
dc.title | Efficient and stable organic solar cells enabled by multicomponent photoactive layer based on one-pot polymerization | - |
dc.type | Article | - |
dc.identifier.wosid | 001003421000016 | - |
dc.identifier.scopusid | 2-s2.0-85148721658 | - |
dc.type.rims | ART | - |
dc.citation.volume | 14 | - |
dc.citation.issue | 1 | - |
dc.citation.publicationname | NATURE COMMUNICATIONS | - |
dc.identifier.doi | 10.1038/s41467-023-36413-3 | - |
dc.contributor.localauthor | Kim, Bumjoon J. | - |
dc.contributor.nonIdAuthor | Liu, Bin | - |
dc.contributor.nonIdAuthor | Sun, Huiliang | - |
dc.contributor.nonIdAuthor | Jiang, Zhengyan | - |
dc.contributor.nonIdAuthor | Qiao, Junqin | - |
dc.contributor.nonIdAuthor | Wang, Junwei | - |
dc.contributor.nonIdAuthor | Yang, Jie | - |
dc.contributor.nonIdAuthor | Feng, Kui | - |
dc.contributor.nonIdAuthor | Liao, Qiaogan | - |
dc.contributor.nonIdAuthor | An, Mingwei | - |
dc.contributor.nonIdAuthor | Li, Bolin | - |
dc.contributor.nonIdAuthor | Han, Dongxue | - |
dc.contributor.nonIdAuthor | Xu, Baomin | - |
dc.contributor.nonIdAuthor | Lian, Hongzhen | - |
dc.contributor.nonIdAuthor | Niu, Li | - |
dc.contributor.nonIdAuthor | Guo, Xugang | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordPlus | ACCEPTOR BLOCK-COPOLYMER | - |
dc.subject.keywordPlus | THERMAL-STABILITY | - |
dc.subject.keywordPlus | ALL-POLYMER | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | MICROSTRUCTURE | - |
dc.subject.keywordPlus | MORPHOLOGY | - |
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