DC Field | Value | Language |
---|---|---|
dc.contributor.author | Jeong, Uiseok | ko |
dc.contributor.author | Kim, HyeonJi | ko |
dc.contributor.author | Ramesh, Sreerangappa | ko |
dc.contributor.author | Dogan, Nesibe A. | ko |
dc.contributor.author | Wongwilawan, Sirinapa | ko |
dc.contributor.author | Kang, Sungsu | ko |
dc.contributor.author | Park, Jungwon | ko |
dc.contributor.author | Cho, Eun Seon | ko |
dc.contributor.author | Yavuz, Cafer T. | ko |
dc.date.accessioned | 2021-10-11T05:30:08Z | - |
dc.date.available | 2021-10-11T05:30:08Z | - |
dc.date.created | 2021-09-24 | - |
dc.date.created | 2021-09-24 | - |
dc.date.created | 2021-09-24 | - |
dc.date.created | 2021-09-24 | - |
dc.date.issued | 2021-10 | - |
dc.identifier.citation | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.60, no.41, pp.22478 - 22486 | - |
dc.identifier.issn | 1433-7851 | - |
dc.identifier.uri | http://hdl.handle.net/10203/288144 | - |
dc.description.abstract | Ordered mesoporous carbon materials offer robust network of organized pores for energy storage and catalysis applications, but suffer from time-consuming and intricate preparations hindering their widespread use. Here we report a new and rapid synthetic route for a N-doped ordered mesoporous carbon structure through a preferential heating of iron oxide nanoparticles by microwaves. A nanoporous covalent organic polymer is first formed in situ covering the hard templates of assembled nanoparticles, paving the way for a long-range order in a carbonaceous nanocomposite precursor. Upon removal of the template, a well-defined cubic mesoporous carbon structure was revealed. The ordered mesoporous carbon was used in solid state hydrogen storage as a host scaffold for NaAlH4, where remarkable improvement in hydrogen desorption kinetics was observed. The state-of-the-art lowest activation energy of dehydrogenation as a single step was attributed to their ordered pore structure and N-doping effect. | - |
dc.language | English | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Rapid Access to Ordered Mesoporous Carbons for Chemical Hydrogen Storage | - |
dc.type | Article | - |
dc.identifier.wosid | 000693214000001 | - |
dc.identifier.scopusid | 2-s2.0-85114346254 | - |
dc.type.rims | ART | - |
dc.citation.volume | 60 | - |
dc.citation.issue | 41 | - |
dc.citation.beginningpage | 22478 | - |
dc.citation.endingpage | 22486 | - |
dc.citation.publicationname | ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | - |
dc.identifier.doi | 10.1002/anie.202109215 | - |
dc.embargo.liftdate | 9999-12-31 | - |
dc.embargo.terms | 9999-12-31 | - |
dc.contributor.localauthor | Cho, Eun Seon | - |
dc.contributor.localauthor | Yavuz, Cafer T. | - |
dc.contributor.nonIdAuthor | Kim, HyeonJi | - |
dc.contributor.nonIdAuthor | Ramesh, Sreerangappa | - |
dc.contributor.nonIdAuthor | Dogan, Nesibe A. | - |
dc.contributor.nonIdAuthor | Kang, Sungsu | - |
dc.contributor.nonIdAuthor | Park, Jungwon | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordAuthor | hard template synthesis | - |
dc.subject.keywordAuthor | hydrogen storage | - |
dc.subject.keywordAuthor | microwave heating | - |
dc.subject.keywordAuthor | nanoconfinement | - |
dc.subject.keywordAuthor | nitrogen doped carbon | - |
dc.subject.keywordPlus | POROUS CARBON | - |
dc.subject.keywordPlus | NITROGEN | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | SIZE | - |
dc.subject.keywordPlus | NANOSTRUCTURES | - |
dc.subject.keywordPlus | NANOPARTICLES | - |
dc.subject.keywordPlus | DECOMPOSITION | - |
dc.subject.keywordPlus | MORPHOLOGY | - |
dc.subject.keywordPlus | FRAMEWORKS | - |
dc.subject.keywordPlus | GRAPHENE | - |
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