Hierarchical Self-Assembly of Perylene Diimide (PDI) Crystals

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dc.contributor.authorKim, Yong-Jaeko
dc.contributor.authorLee, Yongheeko
dc.contributor.authorPark, Kanghoko
dc.contributor.authorAhn, Chi Wonko
dc.contributor.authorJung, Hee-Taeko
dc.contributor.authorJeon, Hwan-Jinko
dc.date.accessioned2021-03-26T03:17:18Z-
dc.date.available2021-03-26T03:17:18Z-
dc.date.created2020-06-23-
dc.date.issued2020-05-
dc.identifier.citationJOURNAL OF PHYSICAL CHEMISTRY LETTERS, v.11, no.10, pp.3934 - 3940-
dc.identifier.issn1948-7185-
dc.identifier.urihttp://hdl.handle.net/10203/282039-
dc.description.abstractControlling molecular self-assembly of organic semiconductors is a key factor in enhancing the performance of organic electronics and optoelectronics. However, unlike various p-type organic semiconductors, it has proven elusive to control molecular self-assembly with about tens of nm dimensions using n-type organic semiconductors including perylene diimide (PDI), which is the most promising alternative to fullerene derivatives, without using an additional synthetic method or additives, thus far. Here, we developed a simple self-assembling method for the hierarchical self-assembly of PDI crystals with nanometer-to-micrometer scale features using pristine PDI-C8 without using an additional synthetic method or additive. Interestingly, we observed crystalline and optical properties of self-assembled PDI crystals depending on their size and structural features. In addition, we fabricated p-n junctions composed of PDI and poly(3-hexylthiophene) (P3HT), where the p-n junctions had coassembled and blended nanomorphologies, and confirmed that coassembled nanomorphologies enabled more effective energy transfer than the blended nanomorphologies.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleHierarchical Self-Assembly of Perylene Diimide (PDI) Crystals-
dc.typeArticle-
dc.identifier.wosid000537432500027-
dc.identifier.scopusid2-s2.0-85085265993-
dc.type.rimsART-
dc.citation.volume11-
dc.citation.issue10-
dc.citation.beginningpage3934-
dc.citation.endingpage3940-
dc.citation.publicationnameJOURNAL OF PHYSICAL CHEMISTRY LETTERS-
dc.identifier.doi10.1021/acs.jpclett.0c01226-
dc.contributor.localauthorJung, Hee-Tae-
dc.contributor.nonIdAuthorLee, Yonghee-
dc.contributor.nonIdAuthorAhn, Chi Won-
dc.contributor.nonIdAuthorJeon, Hwan-Jin-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusFIELD-EFFECT TRANSISTORS-
dc.subject.keywordPlusHIGH-PERFORMANCE-
dc.subject.keywordPlusGROWTH-
dc.subject.keywordPlusWATER-
dc.subject.keywordPlusNANOSTRUCTURES-
dc.subject.keywordPlusSEMICONDUCTOR-
dc.subject.keywordPlusNANOWIRES-
dc.subject.keywordPlusFIBERS-
dc.subject.keywordPlusMOLECULES-
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