DC Field | Value | Language |
---|---|---|
dc.contributor.author | Lee, Jeong-Chan | ko |
dc.contributor.author | Kim, Jin-Oh | ko |
dc.contributor.author | Lee, Ho-Jun | ko |
dc.contributor.author | Shin, Byungha | ko |
dc.contributor.author | Park, Steve | ko |
dc.date.accessioned | 2019-10-15T02:20:06Z | - |
dc.date.available | 2019-10-15T02:20:06Z | - |
dc.date.created | 2019-10-14 | - |
dc.date.created | 2019-10-14 | - |
dc.date.issued | 2019-09 | - |
dc.identifier.citation | CHEMISTRY OF MATERIALS, v.31, no.18, pp.7377 - 7385 | - |
dc.identifier.issn | 0897-4756 | - |
dc.identifier.uri | http://hdl.handle.net/10203/267980 | - |
dc.description.abstract | Herein, meniscus-guided crystallization is introduced as a means to grow high quality metal organic framework (MOF) thin films. A meniscus was formed between a target substrate and a coating blade, and by adjusting various parameters such as substrate temperature and coating speed, supersaturation was precisely controlled, through which the crystallization process was finely tuned. Consequently, a densely packed intergrown MOF thin film with thickness tunability down to 450 nm was demonstrated. The individual crystals exhibited monodispersity in size. Interestingly, the use of a microstructured coating blade resulted in the change of crystal shape, attributed to the supersaturation-induced kinetically driven crystallization proc-ess. Our film growth process is large-area scalable, uses a miniscule amount of solution, and has substrate versatility. Such an insight and demonstration of MOF thin-film growth via meniscus-guided crystallization will be highly useful for the development of various MOF thin-film-based devices in the future. | - |
dc.language | English | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.title | Meniscus-Guided Control of Supersaturation for the Crystallization of High Quality Metal Organic Framework Thin Films | - |
dc.type | Article | - |
dc.identifier.wosid | 000487859200030 | - |
dc.identifier.scopusid | 2-s2.0-85072891995 | - |
dc.type.rims | ART | - |
dc.citation.volume | 31 | - |
dc.citation.issue | 18 | - |
dc.citation.beginningpage | 7377 | - |
dc.citation.endingpage | 7385 | - |
dc.citation.publicationname | CHEMISTRY OF MATERIALS | - |
dc.identifier.doi | 10.1021/acs.chemmater.9b01996 | - |
dc.contributor.localauthor | Shin, Byungha | - |
dc.contributor.localauthor | Park, Steve | - |
dc.contributor.nonIdAuthor | Lee, Ho-Jun | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordPlus | LARGE-AREA | - |
dc.subject.keywordPlus | SHAPE CONTROL | - |
dc.subject.keywordPlus | ADSORPTION | - |
dc.subject.keywordPlus | DEPOSITION | - |
dc.subject.keywordPlus | CRYSTALS | - |
dc.subject.keywordPlus | SURFACES | - |
dc.subject.keywordPlus | DOMAINS | - |
dc.subject.keywordPlus | GROWTH | - |
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