DC Field | Value | Language |
---|---|---|
dc.contributor.author | Lemke, Henrik T. | ko |
dc.contributor.author | Bressler, Christian | ko |
dc.contributor.author | Chen, Lin X. | ko |
dc.contributor.author | Fritz, David M. | ko |
dc.contributor.author | Gaffney, Kelly J. | ko |
dc.contributor.author | Galler, Andreas | ko |
dc.contributor.author | Gawelda, Wojciech | ko |
dc.contributor.author | Haldrup, Kristoffer | ko |
dc.contributor.author | Hartsock, Robert W. | ko |
dc.contributor.author | Ihee, Hyotcherl | ko |
dc.contributor.author | Kim, Jeongho | ko |
dc.contributor.author | Kim, Kyung Hwan | ko |
dc.contributor.author | Lee, Jae Hyuk | ko |
dc.contributor.author | Nielsen, Martin M. | ko |
dc.contributor.author | Stickrath, Andrew B. | ko |
dc.contributor.author | Zhang, Wenkai | ko |
dc.contributor.author | Zhu, Diling | ko |
dc.contributor.author | Cammarata, Marco | ko |
dc.date.accessioned | 2019-03-07T09:32:56Z | - |
dc.date.available | 2019-03-07T09:32:56Z | - |
dc.date.created | 2013-03-18 | - |
dc.date.issued | 2013-01 | - |
dc.identifier.citation | JOURNAL OF PHYSICAL CHEMISTRY A, v.117, no.4, pp.735 - 740 | - |
dc.identifier.issn | 1089-5639 | - |
dc.identifier.uri | http://hdl.handle.net/10203/250873 | - |
dc.description.abstract | X-ray free electron lasers (XFELs) deliver short (<100 fs) and intense (similar to 10(12) photons) pulses of hard X-rays, making them excellent sources for time-resolved studies. Here we show that, despite the inherent instabilities of current (SASE based) XFELs, they can be used for measuring high-quality X-ray absorption data and we report femtosecond time-resolved X-ray absorption near-edge spectroscopy (XANES) measurements of a spin-crossover system, iron(II) tris(2,2'-bipyridine) in water. The data indicate that the low-spin to high-spin transition can be modeled by single-exponential kinetics convoluted with the overall time resolution. The resulting time constant is similar to 160 fs. | - |
dc.language | English | - |
dc.publisher | AMER CHEMICAL SOC | - |
dc.subject | STRUCTURAL DYNAMICS | - |
dc.subject | EXCITED-STATES | - |
dc.subject | COMPLEXES | - |
dc.subject | DIFFRACTION | - |
dc.subject | RELAXATION | - |
dc.subject | IRON(II) | - |
dc.subject | SYSTEMS | - |
dc.subject | SOLIDS | - |
dc.subject | BOND | - |
dc.title | Femtosecond X-ray Absorption Spectroscopy at a Hard X-ray Free Electron Laser: Application to Spin Crossover Dynamics | - |
dc.type | Article | - |
dc.identifier.wosid | 000314492900005 | - |
dc.identifier.scopusid | 2-s2.0-84874204283 | - |
dc.type.rims | ART | - |
dc.citation.volume | 117 | - |
dc.citation.issue | 4 | - |
dc.citation.beginningpage | 735 | - |
dc.citation.endingpage | 740 | - |
dc.citation.publicationname | JOURNAL OF PHYSICAL CHEMISTRY A | - |
dc.identifier.doi | 10.1021/jp312559h | - |
dc.contributor.localauthor | Ihee, Hyotcherl | - |
dc.contributor.nonIdAuthor | Lemke, Henrik T. | - |
dc.contributor.nonIdAuthor | Bressler, Christian | - |
dc.contributor.nonIdAuthor | Chen, Lin X. | - |
dc.contributor.nonIdAuthor | Fritz, David M. | - |
dc.contributor.nonIdAuthor | Gaffney, Kelly J. | - |
dc.contributor.nonIdAuthor | Galler, Andreas | - |
dc.contributor.nonIdAuthor | Gawelda, Wojciech | - |
dc.contributor.nonIdAuthor | Haldrup, Kristoffer | - |
dc.contributor.nonIdAuthor | Hartsock, Robert W. | - |
dc.contributor.nonIdAuthor | Kim, Jeongho | - |
dc.contributor.nonIdAuthor | Kim, Kyung Hwan | - |
dc.contributor.nonIdAuthor | Lee, Jae Hyuk | - |
dc.contributor.nonIdAuthor | Nielsen, Martin M. | - |
dc.contributor.nonIdAuthor | Stickrath, Andrew B. | - |
dc.contributor.nonIdAuthor | Zhang, Wenkai | - |
dc.contributor.nonIdAuthor | Zhu, Diling | - |
dc.contributor.nonIdAuthor | Cammarata, Marco | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordPlus | STRUCTURAL DYNAMICS | - |
dc.subject.keywordPlus | EXCITED-STATES | - |
dc.subject.keywordPlus | COMPLEXES | - |
dc.subject.keywordPlus | DIFFRACTION | - |
dc.subject.keywordPlus | RELAXATION | - |
dc.subject.keywordPlus | IRON(II) | - |
dc.subject.keywordPlus | SYSTEMS | - |
dc.subject.keywordPlus | SOLIDS | - |
dc.subject.keywordPlus | BOND | - |
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