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College of Natural Sciences(자연과학대학)Dept. of Chemistry(화학과)CH-Journal Papers(저널논문)

Ir(III)-Catalyzed Stereoselective Haloamidation of Alkynes Enabled by Ligand Participation

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dc.contributor.authorHong, Seung Younko
dc.contributor.authorSon, Junsooko
dc.contributor.authorKim, Dongwookko
dc.contributor.authorChang, Sukbokko
dc.date.accessioned2018-11-12T04:52:25Z-
dc.date.available2018-11-12T04:52:25Z-
dc.date.created2018-10-29-
dc.date.created2018-10-29-
dc.date.issued2018-10-
dc.identifier.citationJOURNAL OF THE AMERICAN CHEMICAL SOCIETY, v.140, no.39, pp.12359 - 12363-
dc.identifier.issn0002-7863-
dc.identifier.urihttp://hdl.handle.net/10203/246568-
dc.description.abstractDescribed herein is the application of a strategy of ligand participation for the Ir-catalyzed imido transfer into alkynes. On the basis of a stoichiometric [3 + 2] cycloaddition of Cp*Ir(III)(kappa(2)-N,O-chelate) with alkynyl dioxazolone, a catalytic haloamidation was developed for the first time by employing [Cp*IrCl2](2) precatalyst and NaX salts (X = Cl or Br) as practical halide sources to furnish synthetically versatile Z-(halovinyl)lactams with excellent stereoselectivity.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.subjectC-H AMIDATION-
dc.subjectCOUPLING REACTIONS-
dc.subjectCASCADE REACTIONS-
dc.subjectVINYL CHLORIDES-
dc.subjectAMIDO TRANSFER-
dc.subjectAMINATION-
dc.subjectMILD-
dc.subjectFUNCTIONALIZATION-
dc.subjectDIOXAZOLONES-
dc.subjectCOMPLEXES-
dc.titleIr(III)-Catalyzed Stereoselective Haloamidation of Alkynes Enabled by Ligand Participation-
dc.typeArticle-
dc.identifier.wosid000446920100012-
dc.identifier.scopusid2-s2.0-85053848161-
dc.type.rimsART-
dc.citation.volume140-
dc.citation.issue39-
dc.citation.beginningpage12359-
dc.citation.endingpage12363-
dc.citation.publicationnameJOURNAL OF THE AMERICAN CHEMICAL SOCIETY-
dc.identifier.doi10.1021/jacs.8b08134-
dc.contributor.localauthorChang, Sukbok-
dc.contributor.nonIdAuthorKim, Dongwook-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusC-H AMIDATION-
dc.subject.keywordPlusCOUPLING REACTIONS-
dc.subject.keywordPlusCASCADE REACTIONS-
dc.subject.keywordPlusVINYL CHLORIDES-
dc.subject.keywordPlusAMIDO TRANSFER-
dc.subject.keywordPlusAMINATION-
dc.subject.keywordPlusMILD-
dc.subject.keywordPlusFUNCTIONALIZATION-
dc.subject.keywordPlusDIOXAZOLONES-
dc.subject.keywordPlusCOMPLEXES-
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