DC Field | Value | Language |
---|---|---|
dc.contributor.author | Lei, Ting | ko |
dc.contributor.author | Pitner, Gregory | ko |
dc.contributor.author | Chen, Xiyuan | ko |
dc.contributor.author | Hong, Guosong | ko |
dc.contributor.author | Park, Steve | ko |
dc.contributor.author | Hayoz, Pascal | ko |
dc.contributor.author | Weitz, Ralf Thomas | ko |
dc.contributor.author | Wong, Hon Sum Philip | ko |
dc.contributor.author | Bao, Zhenan | ko |
dc.date.accessioned | 2017-01-13T05:08:56Z | - |
dc.date.available | 2017-01-13T05:08:56Z | - |
dc.date.created | 2016-02-23 | - |
dc.date.created | 2016-02-23 | - |
dc.date.created | 2016-02-23 | - |
dc.date.issued | 2016-01 | - |
dc.identifier.citation | ADVANCED ELECTRONIC MATERIALS, v.2, no.1 | - |
dc.identifier.issn | 2199-160X | - |
dc.identifier.uri | http://hdl.handle.net/10203/218773 | - |
dc.description.abstract | The isolation of semiconducting single-walled carbon nanotubes (sc-SWNTs) with ideal diameter and high purity is highly desired for high-performance electronic devices. However, current sorting methods for large-diameter sc-SWNTs suffer from either low purity (<99%) or long processing time (>20 h). Here, a backbone-engineering strategy is reported for the polymer used for sorting to improve the purity of sorted sc-SWNTs. Six diketopyrrolopyrrole (DPP)-based conjugated polymers are used to systematically investigate their sorting ability for sc-SWNTs. It is found that incorporation of more thiophenes building blocks in the repeating units of DPP polymer backbone leads to increased selectivity and yield for sc-SWNTs. The DPP polymers can disperse sc-SWNTs with 1.4-1.6 nm in diameter and high purity of 99.6% by a processing time as short as 1 h. Furthermore, a scalable film coating method named "solution shearing" is used to fabricate SWNT network thin-film transistors (TFTs). The TFT devices exhibit both high mobilities over 50 cm(2) V-1 s(-1) and high on/off ratios over 10(5), which are among the highest performance for solution-processed SWNT network TFTs. | - |
dc.language | English | - |
dc.publisher | WILEY-BLACKWELL | - |
dc.subject | THIN-FILM TRANSISTORS | - |
dc.subject | FIELD-EFFECT TRANSISTORS | - |
dc.subject | SELECTIVE DISPERSION | - |
dc.subject | SINGLE-WALL | - |
dc.subject | SOLAR-CELLS | - |
dc.subject | PERFORMANCE | - |
dc.subject | SEPARATION | - |
dc.subject | QUANTIFICATION | - |
dc.subject | EXTRACTION | - |
dc.subject | TRANSPORT | - |
dc.title | Dispersion of High-Purity Semiconducting Arc-Discharged Carbon Nanotubes Using Backbone Engineered Diketopyrrolopyrrole (DPP)-Based Polymers | - |
dc.type | Article | - |
dc.identifier.wosid | 000370335000018 | - |
dc.identifier.scopusid | 2-s2.0-84995508040 | - |
dc.type.rims | ART | - |
dc.citation.volume | 2 | - |
dc.citation.issue | 1 | - |
dc.citation.publicationname | ADVANCED ELECTRONIC MATERIALS | - |
dc.identifier.doi | 10.1002/aelm.201500299 | - |
dc.contributor.localauthor | Park, Steve | - |
dc.contributor.nonIdAuthor | Lei, Ting | - |
dc.contributor.nonIdAuthor | Pitner, Gregory | - |
dc.contributor.nonIdAuthor | Chen, Xiyuan | - |
dc.contributor.nonIdAuthor | Hong, Guosong | - |
dc.contributor.nonIdAuthor | Hayoz, Pascal | - |
dc.contributor.nonIdAuthor | Weitz, Ralf Thomas | - |
dc.contributor.nonIdAuthor | Wong, Hon Sum Philip | - |
dc.contributor.nonIdAuthor | Bao, Zhenan | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordPlus | THIN-FILM TRANSISTORS | - |
dc.subject.keywordPlus | FIELD-EFFECT TRANSISTORS | - |
dc.subject.keywordPlus | SELECTIVE DISPERSION | - |
dc.subject.keywordPlus | SINGLE-WALL | - |
dc.subject.keywordPlus | SOLAR-CELLS | - |
dc.subject.keywordPlus | PERFORMANCE | - |
dc.subject.keywordPlus | SEPARATION | - |
dc.subject.keywordPlus | QUANTIFICATION | - |
dc.subject.keywordPlus | EXTRACTION | - |
dc.subject.keywordPlus | TRANSPORT | - |
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