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College of Natural Sciences(자연과학대학)Dept. of Chemistry(화학과)CH-Journal Papers(저널논문)

Rh-I-Catalyzed Site-Selective Decarbonylative Alkenylation and Arylation of Quinolones under Chelation Assistance

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dc.contributor.authorKwon, Soonhyungko
dc.contributor.authorKang, Dahyeko
dc.contributor.authorHong, Sung-Wooko
dc.date.accessioned2015-07-01T02:57:11Z-
dc.date.available2015-07-01T02:57:11Z-
dc.date.created2015-06-30-
dc.date.created2015-06-30-
dc.date.issued2015-06-
dc.identifier.citationEUROPEAN JOURNAL OF ORGANIC CHEMISTRY, no.17, pp.3671 - 3678-
dc.identifier.issn1434-193X-
dc.identifier.urihttp://hdl.handle.net/10203/199619-
dc.description.abstractAn efficient catalytic system for the C-2 selective C-H functionalization of 4-quinolones was developed by using a decarbonylative coupling strategy. The installation of an N-pyrimidyl group on the quinolone nitrogen atom redirected the coordination between the catalyst and the carbonyl group to promote direct C-H functionalization at the 2-position of 4-quinolones. In addition, the present protocol was successfully applied to the C-3 selective installation of a variety of aryl and vinyl groups on an isoquinolone scaffold.-
dc.languageEnglish-
dc.publisherWILEY-V C H VERLAG GMBH-
dc.subjectC-H BOND-
dc.subjectPALLADIUM(II)-CATALYZED DIRECT ARYLATION-
dc.subjectRH(I)-CATALYZED DIRECT ARYLATION-
dc.subjectCYCLIC ENAMINONES-
dc.subjectCINNAMIC ANHYDRIDES-
dc.subjectCARBOXYLIC-ACIDS-
dc.subjectANTITUMOR AGENTS-
dc.subjectCYANIDE SOURCE-
dc.subject4-QUINOLONES-
dc.subjectINDOLES-
dc.titleRh-I-Catalyzed Site-Selective Decarbonylative Alkenylation and Arylation of Quinolones under Chelation Assistance-
dc.typeArticle-
dc.identifier.wosid000355534600006-
dc.identifier.scopusid2-s2.0-84934873113-
dc.type.rimsART-
dc.citation.issue17-
dc.citation.beginningpage3671-
dc.citation.endingpage3678-
dc.citation.publicationnameEUROPEAN JOURNAL OF ORGANIC CHEMISTRY-
dc.identifier.doi10.1002/ejoc.201500187-
dc.contributor.localauthorHong, Sung-Woo-
dc.type.journalArticleArticle-
dc.subject.keywordAuthorHomogenous catalysis-
dc.subject.keywordAuthorRhodium-
dc.subject.keywordAuthorC-H functionalization-
dc.subject.keywordAuthorCross-coupling-
dc.subject.keywordAuthorOlefination-
dc.subject.keywordAuthorRegioselectivity-
dc.subject.keywordAuthorNitrogen heterocycles-
dc.subject.keywordPlusC-H BOND-
dc.subject.keywordPlusPALLADIUM(II)-CATALYZED DIRECT ARYLATION-
dc.subject.keywordPlusRH(I)-CATALYZED DIRECT ARYLATION-
dc.subject.keywordPlusCYCLIC ENAMINONES-
dc.subject.keywordPlusCINNAMIC ANHYDRIDES-
dc.subject.keywordPlusCARBOXYLIC-ACIDS-
dc.subject.keywordPlusANTITUMOR AGENTS-
dc.subject.keywordPlusCYANIDE SOURCE-
dc.subject.keywordPlus4-QUINOLONES-
dc.subject.keywordPlusINDOLES-
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