DC Field | Value | Language |
---|---|---|
dc.contributor.author | Lee, Sahng-Ha | ko |
dc.contributor.author | Kim, Jae-Hong | ko |
dc.contributor.author | Park, Chan-Beum | ko |
dc.date.accessioned | 2013-06-07T07:56:56Z | - |
dc.date.available | 2013-06-07T07:56:56Z | - |
dc.date.created | 2013-05-07 | - |
dc.date.created | 2013-05-07 | - |
dc.date.issued | 2013-04 | - |
dc.identifier.citation | CHEMISTRY-A EUROPEAN JOURNAL, v.19, no.14, pp.4392 - 4406 | - |
dc.identifier.issn | 0947-6539 | - |
dc.identifier.uri | http://hdl.handle.net/10203/173786 | - |
dc.description.abstract | In green plants, solar-energy utilization is accomplished through a cascade of photoinduced electron transfer, which remains a target model for realizing artificial photosynthesis. We introduce the concept of biocatalyzed artificial photosynthesis through coupling redox biocatalysis with photocatalysis to mimic natural photosynthesis based on visible-light-driven regeneration of enzyme cofactors. Key design principles for reaction components, such as electron donors, photosensitizers, and electron mediators, are described for artificial photosynthesis involving biocatalytic assemblies. Recent research outcomes that serve as a proof of the concept are summarized and current issues are discussed to provide a future perspective. | - |
dc.language | English | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.subject | PHOTOINDUCED ELECTRON-TRANSFER | - |
dc.subject | VISIBLE-LIGHT IRRADIATION | - |
dc.subject | SOLAR-ENERGY CONVERSION | - |
dc.subject | WATER OXIDATION | - |
dc.subject | ELECTROCHEMICAL REGENERATION | - |
dc.subject | BIOORGANOMETALLIC CHEMISTRY | - |
dc.subject | NONENZYMATIC REGENERATION | - |
dc.subject | REGIOSELECTIVE REDUCTION | - |
dc.subject | PHOTOENZYMATIC SYNTHESIS | - |
dc.subject | NICOTINAMIDE COFACTOR | - |
dc.title | Coupling Photocatalysis and Redox Biocatalysis Toward Biocatalyzed Artificial Photosynthesis | - |
dc.type | Article | - |
dc.identifier.wosid | 000316625000001 | - |
dc.identifier.scopusid | 2-s2.0-84875361540 | - |
dc.type.rims | ART | - |
dc.citation.volume | 19 | - |
dc.citation.issue | 14 | - |
dc.citation.beginningpage | 4392 | - |
dc.citation.endingpage | 4406 | - |
dc.citation.publicationname | CHEMISTRY-A EUROPEAN JOURNAL | - |
dc.identifier.doi | 10.1002/chem.201204385 | - |
dc.contributor.localauthor | Park, Chan-Beum | - |
dc.contributor.nonIdAuthor | Kim, Jae-Hong | - |
dc.type.journalArticle | Review | - |
dc.subject.keywordAuthor | biocatalysis | - |
dc.subject.keywordAuthor | electron transport | - |
dc.subject.keywordAuthor | photocatalysis | - |
dc.subject.keywordAuthor | photosynthesis | - |
dc.subject.keywordAuthor | redox chemistry | - |
dc.subject.keywordPlus | PHOTOINDUCED ELECTRON-TRANSFER | - |
dc.subject.keywordPlus | VISIBLE-LIGHT IRRADIATION | - |
dc.subject.keywordPlus | SOLAR-ENERGY CONVERSION | - |
dc.subject.keywordPlus | WATER OXIDATION | - |
dc.subject.keywordPlus | ELECTROCHEMICAL REGENERATION | - |
dc.subject.keywordPlus | BIOORGANOMETALLIC CHEMISTRY | - |
dc.subject.keywordPlus | NONENZYMATIC REGENERATION | - |
dc.subject.keywordPlus | REGIOSELECTIVE REDUCTION | - |
dc.subject.keywordPlus | PHOTOENZYMATIC SYNTHESIS | - |
dc.subject.keywordPlus | NICOTINAMIDE COFACTOR | - |
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