Nanosphere Templated Continuous PEDOT:PSS Films with Low Percolation Threshold for Application in Efficient Polymer Solar Cells

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dc.contributor.authorKang, Dong Jinko
dc.contributor.authorKang, Hyunbumko
dc.contributor.authorKim, Ki-Hyunko
dc.contributor.authorKim, Bumjoonko
dc.date.accessioned2013-03-12T15:13:40Z-
dc.date.available2013-03-12T15:13:40Z-
dc.date.created2012-11-02-
dc.date.created2012-11-02-
dc.date.issued2012-09-
dc.identifier.citationACS NANO, v.6, no.9, pp.7902 - 7909-
dc.identifier.issn1936-0851-
dc.identifier.urihttp://hdl.handle.net/10203/102681-
dc.description.abstractNanometer-sized monodisperse polystyrene nanospheres (PS NS) were designed as an opal template for the formation of three-dimensionally continuous poly(3,4-ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) films. The resultant films were successfully applied as the anode buffer layer (ABL) to produce highly efficient polymer solar cells (PSCs) with enhanced stability. The conductivity of the PS NS-PEDOT:PSS films was maintained up to phi(PS) = 0.75-0.80, indicating that the formation of continuous PEDOT:PSS films using PS NS templates was successful. To demonstrate the applicability of the PS NS-PEDOT:PSS film for organic electronics, the PS NS-PEDOT:PSS films were used as ABLs in two different PSCs: P3HT:PCBM and P3HT: OXCBA. The photovoltaic performances of both PSCs were maintained up to phi(PS) = 0.8. In particular, the power conversion efficiency of the P3HT:OXCBA PSC with a PS NS-PEDOT:PSS ABL (phi(PS) = 0.8) was greater than 5% and the air stability of the device was significantly enhanced.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.subjectINDIUM-TIN-OXIDE-
dc.subjectCHARGE-TRANSPORT-
dc.subjectPHOTOVOLTAIC CELLS-
dc.subjectBLOCK-COPOLYMERS-
dc.subjectINVERSE OPALS-
dc.subjectBLENDS-
dc.subjectNANOPARTICLES-
dc.subjectPERFORMANCE-
dc.subjectCOLLOIDS-
dc.subjectLAYERS-
dc.titleNanosphere Templated Continuous PEDOT:PSS Films with Low Percolation Threshold for Application in Efficient Polymer Solar Cells-
dc.typeArticle-
dc.identifier.wosid000309040600038-
dc.identifier.scopusid2-s2.0-84866672173-
dc.type.rimsART-
dc.citation.volume6-
dc.citation.issue9-
dc.citation.beginningpage7902-
dc.citation.endingpage7909-
dc.citation.publicationnameACS NANO-
dc.identifier.doi10.1021/nn3022926-
dc.contributor.localauthorKim, Bumjoon-
dc.type.journalArticleArticle-
dc.subject.keywordPlusINDIUM-TIN-OXIDE-
dc.subject.keywordPlusCHARGE-TRANSPORT-
dc.subject.keywordPlusPHOTOVOLTAIC CELLS-
dc.subject.keywordPlusBLOCK-COPOLYMERS-
dc.subject.keywordPlusINVERSE OPALS-
dc.subject.keywordPlusBLENDS-
dc.subject.keywordPlusNANOPARTICLES-
dc.subject.keywordPlusPERFORMANCE-
dc.subject.keywordPlusCOLLOIDS-
dc.subject.keywordPlusLAYERS-
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