Shedding light on biocatalysis: photoelectrochemical platforms for solar-driven biotransformation

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Redox biocatalysis has come to the forefront because of its excellent catalytic efficiency, stereoselectivity, and environmental benignity. The green and sustainable biotransformation can be driven by photoelectrochemical (PEC) platforms where redox biocatalysis is coupled with photoelectrocatalysis. The main challenge is how to transfer photoexcited electrons to (or from) the enzyme redox centers for effective biotransformation using solar energy. This review commences with a conceptual discussion of biocatalytic PEC platforms and highlights recent advances in PEC-based biotransformation through cofactor regeneration or direct transfer of charge carriers to (or from) oxidoreductases on enzyme-conjugated electrodes. Finally, we address future perspectives and potential next steps in the vibrant field of biocatalytic photosynthesis.
Publisher
ELSEVIER SCI LTD
Issue Date
2019-04
Language
English
Article Type
Review
Citation

CURRENT OPINION IN CHEMICAL BIOLOGY, v.49, pp.122 - 129

ISSN
1367-5931
DOI
10.1016/j.cbpa.2018.12.002
URI
http://hdl.handle.net/10203/262218
Appears in Collection
MS-Journal Papers(저널논문)
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