On the Erosion of Enantiopurity of Rhodonoids via Their Asymmetric Total Synthesis

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Rhodonoid natural products are found in nature as a scalemic mixture. This interesting phytochemical feature is presumed to originate from a reversible electrocyclic ring opening of the chromene core present in the biogenetic precursors of rhodonoids. Herein, we systematically investigated factors that are responsible for this racemization event. This eventually led us to complete the asymmetric total synthesis of rhodonoids A, C, D, and G.
Publisher
AMER CHEMICAL SOC
Issue Date
2022-03
Language
English
Article Type
Article
Citation

ORGANIC LETTERS, v.24, no.11, pp.2181 - 2185

ISSN
1523-7060
DOI
10.1021/acs.orglett.2c00482
URI
http://hdl.handle.net/10203/292751
Appears in Collection
CH-Journal Papers(저널논문)
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