DC Field | Value | Language |
---|---|---|
dc.contributor.author | Mahato, Manmatha | ko |
dc.contributor.author | Nam, Sanghee | ko |
dc.contributor.author | Tabassian, Rassoul | ko |
dc.contributor.author | Oh, Saewoong | ko |
dc.contributor.author | Nguyen, Van Hiep | ko |
dc.contributor.author | Oh, Il-Kwon | ko |
dc.date.accessioned | 2022-02-08T06:48:28Z | - |
dc.date.available | 2022-02-08T06:48:28Z | - |
dc.date.created | 2021-10-14 | - |
dc.date.created | 2021-10-14 | - |
dc.date.created | 2021-10-14 | - |
dc.date.issued | 2022-01 | - |
dc.identifier.citation | ADVANCED FUNCTIONAL MATERIALS, v.32, no.5 | - |
dc.identifier.issn | 1616-301X | - |
dc.identifier.uri | http://hdl.handle.net/10203/292164 | - |
dc.description.abstract | Multifunctional porous carbon materials are the key to a clean, safe, and sustainable working environment and energy storage devices because they can be reused, recycled, and repurposed. Here, unprecedented electronically conjugated nanoporous covalent triazine frameworks (CTFs) containing 4-(Dicyanomethylene)-2,6-dimethyl-4H-pyran (DDP) surface functionalities is designed for the selective adsorption of carbon dioxide (CO2) over nitrogen (N-2) gas under ambient conditions; materials are repurposed to form an active electrode material for the fabrication of dimensionally stable high energy density solid-state flexible supercapacitors (SFSC). The functional 4H-pyran unit of DDP in-resonance with the triazine frameworks enriches the overall surface polarities for improved selective gas adsorption and serves as charge storage and/or discharge pockets during electrochemical switching. Consequently, DDP-based CTFs show an optimum CO2 adsorption of 154.0 mg g(-1) and record CO2/N-2 selectivity of 185.8 at 273 K under atmospheric pressure. In addition, an eminent energy density of 147.5 Wh kg(-1) at a power density of 750 W kg(-1) is accomplished with the fabricated SFSC. This material demonstrates no loss of capacitive performance under mechanical bending of 140 degrees for long cycles and can power a commercial light emitting diode easily. | - |
dc.language | English | - |
dc.publisher | WILEY-V C H VERLAG GMBH | - |
dc.title | Electronically Conjugated Multifunctional Covalent Triazine Framework for Unprecedented CO2 Selectivity and High-Power Flexible Supercapacitor | - |
dc.type | Article | - |
dc.identifier.wosid | 000709829100001 | - |
dc.identifier.scopusid | 2-s2.0-85117485276 | - |
dc.type.rims | ART | - |
dc.citation.volume | 32 | - |
dc.citation.issue | 5 | - |
dc.citation.publicationname | ADVANCED FUNCTIONAL MATERIALS | - |
dc.identifier.doi | 10.1002/adfm.202107442 | - |
dc.contributor.localauthor | Oh, Il-Kwon | - |
dc.contributor.nonIdAuthor | Mahato, Manmatha | - |
dc.description.isOpenAccess | N | - |
dc.type.journalArticle | Article | - |
dc.subject.keywordAuthor | 4-(dicyanomethylene)-2 | - |
dc.subject.keywordAuthor | 6-dimethyl-4H-pyran | - |
dc.subject.keywordAuthor | CO | - |
dc.subject.keywordAuthor | (2) adsorption | - |
dc.subject.keywordAuthor | CO | - |
dc.subject.keywordAuthor | (2) | - |
dc.subject.keywordAuthor | N | - |
dc.subject.keywordAuthor | (2) selectivity | - |
dc.subject.keywordAuthor | covalent triazine frameworks | - |
dc.subject.keywordAuthor | multifunctional carbon materials | - |
dc.subject.keywordAuthor | solid-state flexible supercapacitors | - |
dc.subject.keywordPlus | ORGANIC FRAMEWORKS | - |
dc.subject.keywordPlus | GAS-ADSORPTION | - |
dc.subject.keywordPlus | ENERGY DENSITY | - |
dc.subject.keywordPlus | CARBON | - |
dc.subject.keywordPlus | NITROGEN | - |
dc.subject.keywordPlus | ELECTROLYTE | - |
dc.subject.keywordPlus | CAPTURE | - |
dc.subject.keywordPlus | CAPACITANCE | - |
dc.subject.keywordPlus | TEMPERATURE | - |
dc.subject.keywordPlus | ACTIVATION | - |
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