Experimental Observation of the Autler-Townes Splitting in Polyatomic Molecules

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dc.contributor.authorKim, Junggilko
dc.contributor.authorLim, Jean Sunko
dc.contributor.authorNoh, Heung-Ryoulko
dc.contributor.authorKim, Sang Kyuko
dc.date.accessioned2021-03-26T02:30:36Z-
dc.date.available2021-03-26T02:30:36Z-
dc.date.created2020-09-21-
dc.date.issued2020-08-
dc.identifier.citationJOURNAL OF PHYSICAL CHEMISTRY LETTERS, v.11, no.16, pp.6791 - 6795-
dc.identifier.issn1948-7185-
dc.identifier.urihttp://hdl.handle.net/10203/281931-
dc.description.abstractAutler-Townes (AT) splitting has been experimentally observed in the optical transition between the zero-point levels of S-1 and S(0 )for supersonically cooled 2-methoxythiophenol, 2-fluorothiophenol, and 2-chlorothiophenol. This is the first experimental observation of the light-dressed quantum states of polyatomic molecules (N > 3) in the electronic transition. In the resonance-enhanced ionization process involving the optically coupled states, if Rabi cycling is ensured within the nanosecond laser pulse, AT splitting is clearly observed for the open system for which the excited-state lifetime is shorter than hundreds of picoseconds. Semiclassical optical Bloch equations and a dressed-atom approach based on the three-level atomic model describe the experiment quite well, giving deep insights into the light-matter interaction in polyatomic molecular systems.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleExperimental Observation of the Autler-Townes Splitting in Polyatomic Molecules-
dc.typeArticle-
dc.identifier.wosid000563737900047-
dc.identifier.scopusid2-s2.0-85089768685-
dc.type.rimsART-
dc.citation.volume11-
dc.citation.issue16-
dc.citation.beginningpage6791-
dc.citation.endingpage6795-
dc.citation.publicationnameJOURNAL OF PHYSICAL CHEMISTRY LETTERS-
dc.identifier.doi10.1021/acs.jpclett.0c01918-
dc.contributor.localauthorKim, Sang Kyu-
dc.contributor.nonIdAuthorNoh, Heung-Ryoul-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusOPTICAL DOUBLE-RESONANCE-
dc.subject.keywordPlusDYNAMIC STARK CONTROL-
dc.subject.keywordPlusMULTIPHOTON IONIZATION-
dc.subject.keywordPlusPHOTODISSOCIATION-
dc.subject.keywordPlusSPECTROSCOPY-
dc.subject.keywordPlusTRANSITION-
dc.subject.keywordPlusSPECTRA-
dc.subject.keywordPlus2-COLOR-
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