Versatile Processing of Metal-Organic Framework-Fluoropolymer Composite Inks with Chemical Resistance and Sensor Applications

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We report a new class of metal-organic framework (MOF) inks with a water-repellent, photocurable fluoropolyrner (PFPE) having up to 90 wt % MOF loading. These MOF inks are enabled to process various MOFs through spray coating, pen writing, stencil printing, and molding at room temperature. Upon UV curing, the hydrophobic PFPE matrix efficiently blocks water permeation but allows accessibility of chemicals into the MOF pores, thereby freeing the MOF to perform its unique function. Moreover, by introducing functional MOFs we successfully demonstrated a water-tolerant chemosensor for a class of aromatic pollutants in water and a chemical-resistant thermosensor for visualizing temperature image. This approach would open up innumerable opportunities for those MOFs that are otherwise dormant.
Publisher
AMER CHEMICAL SOC
Issue Date
2019-01
Language
English
Article Type
Article
Citation

ACS APPLIED MATERIALS & INTERFACES, v.11, no.4, pp.4385 - 4392

ISSN
1944-8244
DOI
10.1021/acsami.8b19630
URI
http://hdl.handle.net/10203/250492
Appears in Collection
MS-Journal Papers(저널논문)
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