Molecular tuning of amino acids to form two-dimensional molecular networks driven by conformational preorganization

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We investigated the self-assembly of rationally designed gamma-Phe on Au(111) using scanning tunneling microscopy with density functional theory calculations. In contrast to alpha-Phe, gamma-Phe self-assembled into ring-shaped clusters (RSCs) and two-dimensional (2D) molecular domains. The better self-association tendency was attributed to conformational preorganization through intramolecular interaction between ammonium and carboxylate functionalities.
Publisher
ROYAL SOC CHEMISTRY
Issue Date
2016
Language
English
Article Type
Article
Keywords

SCANNING-TUNNELING-MICROSCOPY; L-CYSTEINE; CHIRAL ORGANIZATION; L-METHIONINE; AU(111); BETA; ADSORPTION; PEPTIDES; DESIGN; NANOSTRUCTURES

Citation

CHEMICAL COMMUNICATIONS, v.52, no.97, pp.14055 - 14058

ISSN
1359-7345
DOI
10.1039/c6cc05497h
URI
http://hdl.handle.net/10203/220226
Appears in Collection
CH-Journal Papers(저널논문)
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