Hydrogen-Bonding-Assisted Ketimine Formation of Benzophenone Derivatives

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dc.contributor.authorSeo, Min Seobko
dc.contributor.authorJang, Suminko
dc.contributor.authorJung, Hoiminko
dc.contributor.authorKim, Hyunwooko
dc.date.accessioned2019-01-22T08:30:57Z-
dc.date.available2019-01-22T08:30:57Z-
dc.date.created2018-12-26-
dc.date.created2018-12-26-
dc.date.issued2018-12-
dc.identifier.citationJOURNAL OF ORGANIC CHEMISTRY, v.83, no.23, pp.14300 - 14306-
dc.identifier.issn0022-3263-
dc.identifier.urihttp://hdl.handle.net/10203/249004-
dc.description.abstractThe favorable effect of 2-hydroxyphenyl groups for ketimine formation with benzophenone was demonstrated by combining computational and experimental studies. Although direct imine formation between benzophenone and primary amines is challenging, 2-hydroxybenzophenone or 2,2'-dihydroxybenzophenone was readily used for ketimine formation with various primary alkyl amines and anilines. Measured activation parameters and calculated energy profiles indicated that the 2-hydroxyphenyl group can lower both activation barriers and equilibrium energies by establishing intra-molecular and intermolecular hydrogen-bonding interactions.-
dc.languageEnglish-
dc.publisherAMER CHEMICAL SOC-
dc.titleHydrogen-Bonding-Assisted Ketimine Formation of Benzophenone Derivatives-
dc.typeArticle-
dc.identifier.wosid000452929900008-
dc.identifier.scopusid2-s2.0-85058180352-
dc.type.rimsART-
dc.citation.volume83-
dc.citation.issue23-
dc.citation.beginningpage14300-
dc.citation.endingpage14306-
dc.citation.publicationnameJOURNAL OF ORGANIC CHEMISTRY-
dc.identifier.doi10.1021/acs.joc.8b01908-
dc.contributor.localauthorKim, Hyunwoo-
dc.contributor.nonIdAuthorJung, Hoimin-
dc.description.isOpenAccessN-
dc.type.journalArticleArticle-
dc.subject.keywordPlusBASE-
dc.subject.keywordPlusCOMPLEXES-
dc.subject.keywordPlusCATALYSTS-
dc.subject.keywordPlusPHASE-
dc.subject.keywordPlusION-
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