Directed C-H Activation and Tandem Cross-Coupling Reactions Using Palladium Nanocatalysts with Controlled Oxidation

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Controlled oxidation of palladium nanoparticles provided high-valent Pd-IV oxo-clusters which efficiently promote directed C-H halogenation reactions. In addition, palladium nanoparticles can undergo changes in oxidation states to provide both high-valent PdIV and low-valent Pd-0 species within one system, and thus a tandem reaction of C-H halogenation and cross-coupling (C-N, C-C, and C-S bond formation) was successfully established.
Publisher
WILEY-V C H VERLAG GMBH
Issue Date
2017-06
Language
English
Article Type
Article
Keywords

HETEROGENEOUS CATALYSIS; BOND FUNCTIONALIZATION; REDUCTIVE ELIMINATION; NANOPARTICLES; COMPLEXES; TRANSFORMATIONS; CHEMISTRY; PD(III); REACTOR; SURFACE

Citation

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, v.56, no.24, pp.6952 - 6956

ISSN
1433-7851
DOI
10.1002/anie.201700301
URI
http://hdl.handle.net/10203/224527
Appears in Collection
CH-Journal Papers(저널논문)
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